Multiple exciton generation by a single photon in single-walled carbon nanotubes.
نویسندگان
چکیده
Multiple-exciton generation in single-walled carbon nanotubes is investigated theoretically. We show that multiple excitons can be directly generated by a single photon through resonant coupling with multiexciton states. Further, the theoretically predicted threshold energy for this process is consistent with recent experimental results. Our calculations clarify the elementary processes of multiple-exciton generation in single-walled carbon nanotubes.
منابع مشابه
Probing Exciton Dynamics of Semiconducting Single-Walled Carbon Nanotubes Using Photon Echo Spectroscopy
Three-pulse photon echo peak shifts of single-walled carbon nanotubes were recorded at 975 nm, showing an initial value of 26 fs, a dominant decay time of 59 fs and an oscillatory frequency of 282 cm"'.
متن کاملAll-optical trion generation in single-walled carbon nanotubes.
We present evidence of all-optical trion generation and emission in pristine single-walled carbon nanotubes (SWCNTs). Luminescence spectra, recorded on individual SWCNTs over a large cw excitation intensity range, show trion emission peaks redshifted with respect to the bright exciton peak. Clear chirality dependence is observed for 22 separate SWCNT species, allowing for determination of elect...
متن کاملPhotoinduced spontaneous free-carrier generation in semiconducting single-walled carbon nanotubes.
Strong quantum confinement and low dielectric screening impart single-walled carbon nanotubes with exciton-binding energies substantially exceeding kBT at room temperature. Despite these large binding energies, reported photoluminescence quantum yields are typically low and some studies suggest that photoexcitation of carbon nanotube excitonic transitions can produce free charge carriers. Here ...
متن کاملDirect experimental evidence of exciton-phonon bound states in carbon nanotubes.
We present direct experimental observation of exciton-phonon bound states in the photoluminescence excitation spectra of isolated single-walled carbon nanotubes (SWNT) in aqueous suspension. The photoluminescence excitation spectra from several distinct SWNTs show the presence of at least one sideband related to the tangential modes, lying 0.2 eV above the main absorption or emission peak. Both...
متن کاملObservation of the triplet exciton in EuS-coated single-walled nanotubes.
Photon absorption by carbon nanotubes creates bound electron-hole pairs called excitons, which can exist in spin-polarized triplet or spin-unpolarized singlet configurations. Triplet excitons are optically inactive owing to the weak spin-orbit coupling in nanotubes. This prevents the optical injection of electron spin into nanotubes for spintronic applications and limits the efficiency of photo...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید
ثبت ناماگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید
ورودعنوان ژورنال:
- Physical review letters
دوره 108 22 شماره
صفحات -
تاریخ انتشار 2012